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Chiral Hydrogen-Bond Donor and Gold(I) Cocatalysis Enables Enantioselective Dearomative Spirocyclization of Naphthols

Timur Adrianov, Eric N. Jacobsen

2025Journal of the American Chemical Society8 citationsDOIOpen Access PDF

Abstract

We report the enantioselective gold(I)-catalyzed dearomative spirocyclization of naphthols enabled by the cooperative effect of chiral dual hydrogen-bond donors (HBDs). The reaction affords carbocyclic and heterocyclic spirocycles bearing a quaternary stereocenter with high enantioselectivity (up to 99% enantiomeric excess). Kinetic analysis supports a mode of catalysis wherein two molecules of a monomeric urea cocatalyst activate the neutral gold(I) sulfonate complex via anion abstraction to induce enantioselectivity and rate acceleration in the cyclization reaction. A systematic investigation of ligand effects identified a correlation between the electronic properties of the gold(I) phosphine ligand and the observed enantioselectivity.

Topics & Concepts

ChemistryEnantioselective synthesisStereocenterPhosphineLigand (biochemistry)EnantiomerKinetic resolutionCatalysisCombinatorial chemistryStereochemistryMonomerSulfonateEnantiomeric excessChirality (physics)StereoisomerismChiral ligandMoleculeOrganocatalysisSulfonamideLone pairUreaDihydroxylationMedicinal chemistryOrganic chemistryPolyketideCatalytic Alkyne ReactionsAxial and Atropisomeric Chirality SynthesisAsymmetric Hydrogenation and Catalysis
Chiral Hydrogen-Bond Donor and Gold(I) Cocatalysis Enables Enantioselective Dearomative Spirocyclization of Naphthols | Litcius