Toward Room-Temperature Electrical Control of Magnetic Order in Multiferroic van der Waals Materials
Chengxi Huang, Jian Zhou, Huasheng Sun, Fang Wu, Yusheng Hou, Erjun Kan
Abstract
Electrical control of magnetic order in van der Waals (vdW) two-dimensional (2D) systems is appealing for high-efficiency and low-dissipation nanospintronic devices. For realistic applications, a vdW 2D material with ferromagnetic (FM) and ferroelectric (FE) orders coexisting and strongly coupling at room temperature is urgently needed. Here we present a potential candidate for nonvolatile electric-field control of magnetic orders at room temperature. Using first-principles calculations, we predict the coexistence of room-temperature FM and FE orders in a 2D transition metal carbide, where the spatial distribution of magnetic moments strongly couples with the orientation of out-of-plane electric polarization. Furthermore, an electric-field switching between interfacial FM and ferrimagnetic orders is realizable through constructing a multiferroic vdW heterostructure based on this material. These findings make a significant step toward realizing room-temperature multiferroicity and strong magnetoelectric coupling in 2D materials.