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Fabrication of a Sb<sub>2</sub>MoO<sub>6</sub>/g-C<sub>3</sub>N<sub>4</sub> Photocatalyst for Enhanced RhB Degradation and H<sub>2</sub> Generation

Ying Zhao, Huanxian Shi, Dongyuan Yang, Jun Fan, Xiaoyun Hu, Enzhou Liu

2020The Journal of Physical Chemistry C134 citationsDOI

Abstract

In this work, Sb2MoO6 was applied to the field of photocatalysis and employed to modify g-C3N4 for the first time so as to construct the Sb2MoO6/g-C3N4 heterojunction. Results reveal that 7.5% Sb2MoO6/g-C3N4 showed the best activity during photocatalytic RhB degradation and H2 evolution in water. Rates of RhB degradation and H2 evolution were 6.6 and 5.4 times higher than those of g-C3N4, respectively. According to UV–visible absorption spectra, transient photocurrent curves, photoluminescence spectra, and electrochemical impedance spectra, outstanding performance of 7.5% Sb2MoO6/g-C3N4 was benefited from increases in response of visible light and efficient separation of photogenerated carriers. Furthermore, a possible charge carriers’ transmission route was proposed based on the band gap position and characterization consequence.

Topics & Concepts

PhotocatalysisPhotocurrentPhotoluminescenceMaterials scienceHeterojunctionCharge carrierDegradation (telecommunications)Visible spectrumOptoelectronicsBand gapDielectric spectroscopySpectral lineAbsorption (acoustics)Absorption spectroscopyAnalytical Chemistry (journal)ElectrochemistryChemistryOpticsPhysicsPhysical chemistryTelecommunicationsElectrodeComputer scienceCatalysisBiochemistryChromatographyComposite materialAstronomyAdvanced Photocatalysis TechniquesPerovskite Materials and ApplicationsCovalent Organic Framework Applications