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Acceleration of chronic wound healing by bio-inorganic polyphosphate: <i>In vitro</i> studies and first clinical applications

Hadrian Schepler, Meik Neufurth, Shunfeng Wang, Zhengding She, Heinz C. Schröder, Xiaohong Wang, Wernér E.G. Müller

2021Theranostics41 citationsDOIOpen Access PDF

Abstract

The healing of chronic wounds is impaired by a lack of metabolic energy. In previous studies, we showed that physiological inorganic polyphosphate (polyP) is a generator of metabolic energy by forming ATP as a result of the enzymatic cleavage of the high-energy phosphoanhydride bonds of this polymer. Therefore, in the present study, we investigated whether the administration of polyP can substitute for the energy deficiency in chronic wound healing. Methods: PolyP was incorporated into collagen mats and applied in vitro and to patients in vivo. Results: (i) In vitro studies: Keratinocytes grown in vitro onto the polyP/collagen mats formed long microvilli to guide them to a favorable environment. HUVEC cells responded to polyP/collagen mats with an increased adhesion and migration propensity as well as penetration into the mats. (ii) In vivohuman clinical studies: In a "bench to bedside" process these promising in vitro results were translated from the laboratory into the clinic. In the proof-of-concept application, the engineered polyP/collagen mats were applied to chronic wounds in patients. Those mats impressively accelerated the re-epithelialization rate, with a reduction of the wound area to 65% after 3 weeks and to 36.6% and 22.5% after 6 and 9 weeks, respectively. Complete healing was achieved and no further treatment was necessary. Biopsy samples from the regenerating wound area showed predominantly myofibroblasts. The wound healing process was supported by the use of a polyP containing moisturizing solution.

Topics & Concepts

PolyphosphateIn vitroWound healingChemistryBiomedical engineeringMedicineBiochemistrySurgeryPhosphateWound Healing and Treatmentsbiodegradable polymer synthesis and propertiesCoagulation, Bradykinin, Polyphosphates, and Angioedema
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