Self-crosslinked N-doped carbon dot supported Pd as an efficient catalyst for dehydrogenation of formic acid at room temperature
Zhongxuan Lin, Ouyang Liu, Shuyan Guan, Xinru Zhao, Zhenluo Yuan, Xianyun Liu, Linyan Bian, Yanping Fan, Qiuming Peng, Shumin Han, Baozhong Liu
Abstract
The optimized Pd/CDs-III catalyst shows 100% FA dehydrogenation within 21 min, with a TOF value of 256 h −1 at 298 K. This work provides a powerful guidance for the rational design of active catalysts for dehydrogenation of FA.
Topics & Concepts
DehydrogenationCatalysisFormic acidActive carbonDopingMaterials scienceCarbon fibersRational designInorganic chemistryChemical engineeringChemistryNanotechnologyOrganic chemistryComposite materialWaste managementComposite numberOptoelectronicsEngineeringCarbon dioxide utilization in catalysisMetal-Organic Frameworks: Synthesis and ApplicationsCovalent Organic Framework Applications