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Light scattering from spherical and irregular particles over a wide angular range

Prakash Gautam, Hans Moosmüller, Justin B. Maughan, C. M. Sorensen

2024Aerosol Science and Technology11 citationsDOIOpen Access PDF

Abstract

We present laboratory measurements of angular light scattering intensity for aerosolized, micron-sized, irregularly shaped aluminum oxide (Al 2 O 3 ) abrasive powders with different grit sizes. The measurements were carried out with the scattering angle ranging from 0.32 to 177.6 . First, we demonstrate that the light scattering inferred diameters were in good agreement with the intensity-weighted mean sizes and discuss the importance of intensityweighted size distributions. Second, the wide range of scattering angles motivated us to visualize the same scattering intensity data with three methods: (a) logarithmically versus linear scattering angle h, (b) logarithmically versus the logarithmic magnitude of the scattering wave vector q for forward scattering, the method of Qspace analysis, and (c) logarithmically (last 20 degrees of h) versus linear phase angle (180 h). The combination of these viewpoints yields a comprehensive description of the scattering that corresponds to dividing angular scattering into three regimes: forward-, side-, and backscattering. The light scattering measurements were compared to the Mie scattering calculated for homogenous, spherical particles with the same volume-equivalent size distribution as that of the Al 2 O 3 particles determined with an aerodynamic particle sizer. Experimental and Mie-theory results were well-matched in the forward regime which is clearly shown in Qspace but showed a poor matching in the side and backscattering regimes, as displayed in h-and (180 h) space, respectively.

Topics & Concepts

ScatteringOpticsLight scatteringPhysicsForward scatterBiological small-angle scatteringMie scatteringScattering theoryScattering lengthIntensity (physics)Scattering amplitudeDiscrete dipole approximationComputational physicsMaterials scienceSmall-angle neutron scatteringNeutron scatteringAtmospheric aerosols and cloudsAeolian processes and effectsAtmospheric chemistry and aerosols
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