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Direct Observation of Adhesion and Mechanical Behavior of a Single Poly(lactic-<i>co</i>-glycolic acid) (PLGA) Fiber Using an In Situ Technique for Tissue Engineering

Lihua Lou, Tanaji Paul, Brandon Aguiar, Tyler Dolmetsch, Cheng Zhang, Arvind Agarwal

2022ACS Applied Materials & Interfaces17 citationsDOI

Abstract

-glycolic acid) (PLGA) fiber's load-displacement behavior utilizing the nanoindentation technique coupled with a high-resolution in situ imaging system. It is demonstrated that a maximum force of ∼3 μN in the radial direction and displacement of at least 150% of fiber diameter should be applied to acquire the fiber's macroscopic mechanical properties for tissue engineering. The adhesion behavior of a single fiber is captured using a high-resolution camera. The digital image correlation (DIC) technique is adopted to quantify the adhesion force (∼25 μN) between the fiber and the tip. Adhesion force has also been quantified for the fiber after immersing in phosphate-buffered saline (PBS) to mimic the bioenvironment. A 4-fold increase in adhesion force after PBS treatment was observed due to water penetration and hydrolysis on the fiber's surface. A high similarity between mechanical properties of a single fiber and native tissues (elastic modulus of 10-25 kPa) and superior adhesion force (25-107.25 μN) was observed, which is excellent for promoting cell-matrix communication. Overall, this study examines the mechanics of a single fiber using innovative indentation and imaging processing techniques, disclosing its profound and striking roles in tissue engineering.

Topics & Concepts

PLGAMaterials scienceGlycolic acidIn situAdhesionFiberTissue engineeringLactic acidChemical engineeringComposite materialBiomedical engineeringNanotechnologyPolymer chemistryOrganic chemistryBacteriaNanoparticleChemistryGeneticsMedicineEngineeringBiologyElectrospun Nanofibers in Biomedical ApplicationsBone Tissue Engineering Materialsbiodegradable polymer synthesis and properties
Direct Observation of Adhesion and Mechanical Behavior of a Single Poly(lactic-<i>co</i>-glycolic acid) (PLGA) Fiber Using an In Situ Technique for Tissue Engineering | Litcius