Demonstration of X-ray Thomson scattering as diagnostics for miscibility in warm dense matter
S. Frydrych, Jan Vorberger, N. J. Hartley, A. K. Schuster, Kushal Ramakrishna, A. M. Saunders, Tim van Driel, R. W. Falcone, L. B. Fletcher, Eric Galtier, E. J. Gamboa, S. H. Glenzer, E. Granados, M. J. MacDonald, A. J. Mackinnon, E. E. McBride, Inhyuk Nam, P. Neumayer, A. Pak, K. Voigt, M. Roth, Peihao Sun, D. O. Gericke, T. Döppner, D. Kraus
Abstract
The gas and ice giants in our solar system can be seen as a natural laboratory for the physics of highly compressed matter at temperatures up to thousands of kelvins. In turn, our understanding of their structure and evolution depends critically on our ability to model such matter. One key aspect is the miscibility of the elements in their interiors. Here, we demonstrate the feasibility of X-ray Thomson scattering to quantify the degree of species separation in a 1:1 carbon-hydrogen mixture at a pressure of ~150 GPa and a temperature of ~5000 K. Our measurements provide absolute values of the structure factor that encodes the microscopic arrangement of the particles. From these data, we find a lower limit of [Formula: see text]% of the carbon atoms forming isolated carbon clusters. In principle, this procedure can be employed for investigating the miscibility behaviour of any binary mixture at the high-pressure environment of planetary interiors, in particular, for non-crystalline samples where it is difficult to obtain conclusive results from X-ray diffraction. Moreover, this method will enable unprecedented measurements of mixing/demixing kinetics in dense plasma environments, e.g., induced by chemistry or hydrodynamic instabilities.