Litcius/Paper detail

Desulfonylative Coupling of Alkylsulfones with <i>gem-</i>Difluoroalkenes by Visible-Light Photoredox Catalysis

Masakazu Nambo, Koushik Ghosh, Jacky C.‐H. Yim, Yasuyo Tahara, Naoto Inai, Takeshi Yanai, Cathleen M. Crudden

2022ACS Catalysis41 citationsDOI

Abstract

The desulfonylative radical addition of tertiary alkyl groups to gem-difluoroalkenes by photoredox Ir-catalyst is described. This method exhibits broad substrate scope, affording structurally diverse (E)-fluoroalkene derivatives in a highly stereoselective manner. The resulting (E)-fluoroalkenes were converted into complex fused cyclic compounds by intramolecular cyclization reactions. Control experiments and theoretical calculations are consistent with a single Ir catalyst playing the dual role of generating radical species from sulfones via single electron transfer and mediating Z/E isomerization via energy transfer. A subset of fluoroalkenes provided Z stereoisomers with >90% selectivity, but the same alkenes could also be obtained as E isomers with high selectivity by taking advantage of a secondary Z to E photoisomerization.

Topics & Concepts

IsomerizationPhotoredox catalysisChemistryPhotoisomerizationCatalysisIntramolecular forceSelectivityStereoselectivityPhotochemistrySubstrate (aquarium)AlkylElectron transferCombinatorial chemistryStereochemistryOrganic chemistryPhotocatalysisOceanographyGeologyRadical Photochemical ReactionsSulfur-Based Synthesis TechniquesFluorine in Organic Chemistry
Desulfonylative Coupling of Alkylsulfones with <i>gem-</i>Difluoroalkenes by Visible-Light Photoredox Catalysis | Litcius