Litcius/Paper detail

Measuring the Radius of Gyration and Intrinsic Flexibility of Viral Proteins in Buffer Solution Using Small-Angle X-ray Scattering

Riccardo Funari, Nikhil Bhalla, Luigi Gentile

2022ACS Measurement Science Au33 citationsDOIOpen Access PDF

Abstract

Measuring structural features of proteins dispersed in buffer solution, in contrast to crystal form, is indispensable in understanding morphological characteristics of the biomolecule in a native environment. We report on the structure and apparent viscosity of unfolded α and β variants of SARS-CoV-2 spike proteins dispersed in buffer solutions. The radius of gyration of the β variant is found to be larger than that of the α variant, while the ab initio computation of one of the possible particle-like bodies is consistent with the small-angle X-ray scattering (SAXS) profiles resembling a conformation similar to the three-dimensional structure of the folded state of the corresponding α and β spike variant. However, a smaller radius of gyration with respect to the predicted folded state of 2.4 and 2.7 is observed for both α and β variants, respectively. Our work complements the structural characterization of spike proteins using cryo-electron microscopy techniques. The measurement/analysis discussed here might be useful for quick and cost-effective evaluation of several protein structures, let alone mutated viral proteins, which is useful for drug discovery/development applications.

Topics & Concepts

Radius of gyrationSmall-angle X-ray scatteringGyrationCrystallographyScatteringIntrinsically disordered proteinsBiomoleculeChemical physicsRADIUSSmall-angle scatteringChemistryParticle (ecology)Materials sciencePhysicsNanotechnologyPolymerOpticsGeometryGeologyOceanographyComputer scienceOrganic chemistryMathematicsComputer securityBiochemistryProtein Structure and DynamicsProtein purification and stabilityBacteriophages and microbial interactions