Litcius/Paper detail

Manifestations of Rabi Dynamics in the Photoelectron Energy Spectra at Resonant Two-Photon Ionization of Atom by Intense Short Laser Pulses

N. S. Simonović, D. B. Popović, Andrej Bunjac

2023Atoms17 citationsDOIOpen Access PDF

Abstract

We study the Rabi flopping of the population between the ground and excited 2p states of the hydrogen atom, induced by intense short laser pulses of different shapes and of carrier frequency ω=0.375 a.u. which resonantly couples the two states, and manifestations of this dynamics in the energy spectra of photoelectrons produced in the subsequent ionization of the atom from the excited state. It is found that, for Gaussian, half-Gaussian and rectangular pulses, characterized by the same pulse area, the final populations take the same values and the spectra consist of similar patterns having the same number of peaks and approximately the same separation between the prominent edge (Autler–Townes) peaks. The additional analysis in terms of dressed states showed that the mechanism of formation of multiple-peak structures during the photoionization process is the same regardless of the pulse shape. These facts disprove the hypothesis proposed in earlier studies with Gaussian pulse, that the multiple-peak pattern appears due to dynamic interference of the photoelectrons emitted with a time delay at the rising and falling sides of the pulse, since the hypothesis is not applicable to either a half-Gaussian pulse that has no rising part or a rectangular pulse whose intensity is constant.

Topics & Concepts

PhotoionizationAtomic physicsPhysicsExcited stateIonizationPhotoelectric effectAtom (system on chip)Spectral linePulse (music)PopulationPhotonIonOpticsQuantum mechanicsDetectorEmbedded systemDemographyComputer scienceSociologyLaser-Matter Interactions and ApplicationsAdvanced Chemical Physics StudiesSpectroscopy and Quantum Chemical Studies