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Magnetic-Field Effect as a Tool to Investigate Electron Correlation in Strong-Field Ionization

Kang Lin, Xiang Chen, S. Eckart, Hui Jiang, Alexander Hartung, D. Trabert, K. Fehre, J. Rist, Lothar Schmidt, M. S. Schöffler, T. Jahnke, M. Kunitski, Feng He, R. Dörner

2022Physical Review Letters21 citationsDOI

Abstract

The influence of the magnetic component of the driving electromagnetic field is often neglected when investigating light-matter interaction. We show that the magnetic component of the light field plays an important role in nonsequential double ionization, which serves as a powerful tool to investigate electron correlation. We investigate the magnetic-field effects in double ionization of xenon atoms driven by near-infrared ultrashort femtosecond laser pulses and find that the mean forward shift of the electron momentum distribution in light-propagation direction agrees well with the classical prediction, where no under-barrier or recollisional nondipole enhancement is observed. By extending classical trajectory Monte Carlo simulations beyond the dipole approximation, we reveal that double ionization proceeds via recollision-induced doubly excited states, followed by subsequent sequential over-barrier field ionization of the two electrons. In agreement with this model, the binding energies do not lead to an additional nondipole forward shift of the electrons. Our findings provide a new method to study electron correlation by exploiting the effect of the magnetic component of the electromagnetic field.

Topics & Concepts

PhysicsElectronDouble ionizationIonizationAtomic physicsMagnetic fieldDiscrete dipole approximationDipolePhotoionizationElectronic correlationField (mathematics)FemtosecondQuantum tunnellingLaserCondensed matter physicsIonOpticsQuantum mechanicsPure mathematicsMathematicsLaser-Matter Interactions and ApplicationsQuantum optics and atomic interactionsSpectroscopy and Quantum Chemical Studies