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Sustainable and rapid preparation of nanosized Fe/Ni-pentlandite particles by mechanochemistry

David Tetzlaff, Kevinjeorjios Pellumbi, Daniel M. Baier, Lucas Hoof, Harikumar Shastry Barkur, Mathias Smialkowski, Hatem M.A. Amin, Sven Grätz, Daniel Siegmund, Lars Borchardt, Ulf‐Peter Apfel

2020Chemical Science50 citationsDOIOpen Access PDF

Abstract

250 nm in a single synthetic step from elemental- or sulfidic mixtures. We herein highlight the effects of the milling ball quantity, precursor types and milling time on the product quality. Along this line, Raman spectroscopy as well as temperature/pressure monitoring during the milling processes provide valuable insights into mechanistic differences between the mechanochemical Pn-formation. By employing the obtained Pn-nanosized particles as cathodic electrocatalysts for water splitting in a zero-gap PEM electrolyzer we provide a comprehensive path for a potential sustainable future process involving non-noble metal catalysts.

Topics & Concepts

PentlanditeMaterials scienceBall millBimetallic stripMechanochemistryChemical engineeringRaman spectroscopyCatalysisNanotechnologyMetallurgyMetalPyrrhotiteSulfideChemistryOrganic chemistryOpticsEngineeringPhysicsElectrocatalysts for Energy ConversionAdvanced Thermoelectric Materials and DevicesCopper-based nanomaterials and applications
Sustainable and rapid preparation of nanosized Fe/Ni-pentlandite particles by mechanochemistry | Litcius