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Generation of multiple attosecond sub-bursts in femtosecond pulse trains by long-wavelength driving lasers

Zhiming Yin, Xiangyu Tang, Xuhong Li, Beiyu Wang, Jiaxin Han, C. D. Lin, Cheng Jin

2023Physical review. A/Physical review, A13 citationsDOIOpen Access PDF

Abstract

High-order harmonics generated by a long intense femtosecond laser are known experimentally to create attosecond pulse trains (APTs). In the time domain, an APT consists of a sequence of sharp attosecond bursts that are equally separated by each half optical cycle. Here we show that such well-known features can be modified when a longer wavelength driving laser is used. From our simulations, we show that multiple shorter attosecond sub-bursts exist in the femtosecond pulse train within each half optical cycle and the duration of each sub-burst scales approximately as ${\ensuremath{\lambda}}_{0}^{\ensuremath{-}2}$ with the driving laser wavelength ${\ensuremath{\lambda}}_{0}$. We show that such sub-bursts can be found using quantitative rescattering model for harmonics generated from a single atom, and their origin is due to the interference of the quantum orbits from first two returns of the recombining electron. We further show that such sub-bursts can be phase matched under proper laser focusing condition and the position of the gas cell, thus, such new features should be observable experimentally.

Topics & Concepts

AttosecondFemtosecondPhysicsLaserHarmonicsOpticsWavelengthPulse (music)Femtosecond pulse shapingHigh harmonic generationPhase (matter)LambdaUltrashort pulseAtomic physicsQuantum mechanicsDetectorVoltageLaser-Matter Interactions and ApplicationsAdvanced Fiber Laser TechnologiesSpectroscopy and Quantum Chemical Studies