Litcius/Paper detail

Correlation of Interface Interdiffusion and Skyrmionic Phases

Pamela Costa Carvalho, I. P. Miranda, Jeovani Brandão, Anders Bergman, J. C. Cezar, A. B. Klautau, Helena M. Petrilli

2023Nano Letters13 citationsDOIOpen Access PDF

Abstract

Magnetic skyrmions are prime candidates for the next generation of spintronic devices. Skyrmions and other topological magnetic structures are known to be stabilized by the Dzyaloshinskii-Moriya interaction (DMI) that occurs when the inversion symmetry is broken in thin films. Here, we show by first-principles calculations and atomistic spin dynamics simulations that metastable skyrmionic states can also be found in nominally symmetric multilayered systems. We demonstrate that this is correlated with the large enhancement of the DMI strength due to the presence of local defects. In particular, we find that metastable skyrmions can occur in Pd/Co/Pd multilayers without external magnetic fields and can be stable even near room temperature conditions. Our theoretical findings corroborate with magnetic force microscopy images and X-ray magnetic circular dichroism measurements and highlight the possibility of tuning the intensity of DMI by using interdiffusion at thin film interfaces.

Topics & Concepts

SkyrmionSpintronicsCondensed matter physicsMetastabilityPoint reflectionMaterials scienceMagnetic force microscopeAnnealing (glass)Thin filmPhysicsMagnetizationMagnetic fieldFerromagnetismNanotechnologyQuantum mechanicsComposite materialMagnetic properties of thin filmsPhysics of Superconductivity and MagnetismMagnetic and transport properties of perovskites and related materials