A benzimidazole-linked bimetallic phthalocyanine–porphyrin covalent organic framework synergistically promotes CO<sub>2</sub>electroreduction
Xiaoyu Dong, Fang-Qin Yan, Qian‐You Wang, Pengfei Feng, Ru‐Yi Zou, Shan Wang, Shuang‐Quan Zang
Abstract
A bimetallic phthalocyanine–porphyrin covalent organic framework with benzimidazole linkage was developed as an efficient CO 2 electrocatalyst. Mechanistic studies clarified that a synergistic effect in the CO 2 reduction thermodynamic pathway.
Topics & Concepts
BenzimidazoleBimetallic stripPorphyrinPhthalocyanineCovalent bondElectrocatalystChemistryPhotochemistryCovalent organic frameworkCombinatorial chemistryInorganic chemistryCatalysisOrganic chemistryElectrodeElectrochemistryPhysical chemistryCovalent Organic Framework ApplicationsCO2 Reduction Techniques and CatalystsMetal-Organic Frameworks: Synthesis and Applications