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3D chitosan/GO/ZnO hydrogel with enhanced photocorrosion-resistance and adsorption for efficient removal of typical water-soluble pollutants

Liqiang Zhang, Xueying Li, Simiao Chen, Jie Guan, Yaoguang Guo, Wei Yu

2023Catalysis Communications57 citationsDOIOpen Access PDF

Abstract

With high toxicity and solubility, traditional treatment methods are almost ineffective for treating water-soluble pollutants. In this work, an environmentally friendly chitosan/graphene oxide/zinc oxide (chitosan/GO/ZnO, CGZ) three-dimensional (3D) network structure hydrogel was facilely prepared. The hydrogel with high adsorption improves the mass transfer efficiency of pollutant molecules and blocks the direct contact between ZnO and water, improving the photocorrosion-resistance of traditional ZnO photocatalyst. The 3D hydrogel structure is stable and recyclable, which has a degradation rate of 86.5% after four consecutive experiments. The CGZ hydrogel provides an alternative route for the practical application in removal of other water-soluble pollutants.

Topics & Concepts

AdsorptionPollutantPhotocatalysisChitosanChemical engineeringOxideEnvironmentally friendlyGrapheneChemistryWater treatmentPortable water purificationCatalysisDegradation (telecommunications)Materials scienceMoleculeNanotechnologyOrganic chemistryWaste managementEcologyEngineeringTelecommunicationsComputer scienceBiologyZnO doping and propertiesAdvanced Sensor and Energy Harvesting MaterialsAdvanced Photocatalysis Techniques
3D chitosan/GO/ZnO hydrogel with enhanced photocorrosion-resistance and adsorption for efficient removal of typical water-soluble pollutants | Litcius