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Nickel catalyzed C–S cross coupling of sterically hindered substrates enabled by flexible bidentate phosphines

Ivo H. Lindenmaier, Robert C. Richter, Ivana Fleischer

2024Organic Chemistry Frontiers14 citationsDOIOpen Access PDF

Abstract

The challenging nickel-catalyzed coupling of ortho -substituted aryl triflates with thiols was accomplished by employing a versatile bidentate ligand, capable of decoordination of one phosphorus atom during the deprotonation of thiol.

Topics & Concepts

ChemistryDenticityDeprotonationNickelSteric effectsCatalysisArylThiolLigand (biochemistry)Coupling (piping)Combinatorial chemistryPhotochemistryPolymer chemistryMedicinal chemistryStereochemistryOrganic chemistryCrystal structureBiochemistryMetallurgyMaterials scienceIonReceptorAlkylSulfur-Based Synthesis TechniquesCatalytic C–H Functionalization MethodsChemical Synthesis and Reactions
Nickel catalyzed C–S cross coupling of sterically hindered substrates enabled by flexible bidentate phosphines | Litcius