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Comparative Evaluation of Light‐Driven Catalysis: A Framework for Standardized Reporting of Data**

Dirk Ziegenbalg, Andrea Pannwitz, Sven Rau, Benjamin Dietzek‐Ivanšić, Carsten Streb

2022Angewandte Chemie International Edition72 citationsDOIOpen Access PDF

Abstract

Light-driven homogeneous and heterogeneous catalysis require a complex interplay between light absorption, charge separation, charge transfer, and catalytic turnover. Optical and irradiation parameters as well as reaction engineering aspects play major roles in controlling catalytic performance. This multitude of factors makes it difficult to objectively compare light-driven catalysts and provide an unbiased performance assessment. This Scientific Perspective highlights the importance of collecting and reporting experimental data in homogeneous and heterogeneous light-driven catalysis. A critical analysis of the benefits and limitations of the commonly used experimental indicators is provided. Data collection and reporting according to FAIR principles is discussed in the context of future automated data analysis. The authors propose a minimum dataset as a basis for unified collecting and reporting of experimental data in homogeneous and heterogeneous light-driven catalysis. The community is encouraged to support the future development of this parameter list through an open online repository.

Topics & Concepts

HomogeneousContext (archaeology)Experimental dataComputer scienceData scienceBiochemical engineeringPerspective (graphical)EngineeringPhysicsArtificial intelligenceMathematicsThermodynamicsPaleontologyStatisticsBiologyAdvanced Photocatalysis TechniquesCatalytic Processes in Materials ScienceCaching and Content Delivery