Litcius/Paper detail

Production of a monolithic fuel cell stack with high power density

Stéven Pirou, Belma Talic, Karen Brodersen, Anne Hauch, Henrik Lund Frandsen, Theis Løye Skafte, Åsa Helen Persson, Jens Valdemar Thorvald Høgh, Henrik Henriksen, Maria Navasa, Xing-Yuan Miao, Xanthi Georgolamprou, Søren Preben Vagn Foghmoes, Peter Vang Hendriksen, Eva Ravn Nielsen, Jimmi Nielsen, Anders Christian Wulff, Søren Højgaard Jensen, Philipp Zielke, Anke Hagen

2022Nature Communications88 citationsDOIOpen Access PDF

Abstract

The transportation sector is undergoing a technology shift from internal combustion engines to electric motors powered by secondary Li-based batteries. However, the limited range and long charging times of Li-ion batteries still hinder widespread adoption. This aspect is particularly true in the case of heavy freight and long-range transportation, where solid oxide fuel cells (SOFCs) offer an attractive alternative as they can provide high-efficiency and flexible fuel choices. However, the SOFC technology is mainly used for stationary applications owing to the high operating temperature, low volumetric power density and specific power, and poor robustness towards thermal cycling and mechanical vibrations of conventional ceramic-based cells. Here, we present a metal-based monolithic fuel cell design to overcome these issues. Cost-effective and scalable manufacturing processes are employed for fabrication, and only a single heat treatment is required, as opposed to multiple thermal treatments in conventional SOFC production. The design is optimised through three-dimensional multiphysics modelling, nanoparticle infiltration, and corrosion-mitigating treatments. The monolithic fuel cell stack shows a power density of 5.6 kW/L, thus, demonstrating the potential of SOFC technology for transport applications.

Topics & Concepts

MultiphysicsPower densityMaterials scienceStack (abstract data type)Regenerative fuel cellAutomotive engineeringSolid oxide fuel cellScalabilityFabricationCombustionProcess engineeringComputer scienceInternal combustion engineAnodePower (physics)ElectrodeEngineeringHydrogen fuel enhancementFinite element methodOrganic chemistryChemistryAlternative medicineProgramming languageDatabaseQuantum mechanicsPhysicsPhysical chemistryMedicinePathologyStructural engineeringAdvancements in Solid Oxide Fuel CellsFuel Cells and Related MaterialsElectrocatalysts for Energy Conversion