Litcius/Paper detail

Polarization-Independent Enhancement of Third-Harmonic Generation Empowered by Doubly Degenerate Quasi-Bound States in the Continuum

Tingting Liu, Meibao Qin, Jumin Qiu, Xu Tu, Huifu Qiu, Feng Wu, Tianbao Yu, Qiegen Liu, Shuyuan Xiao

2025Nano Letters70 citationsDOIOpen Access PDF

Abstract

High Resolution Image Download MS PowerPoint Slide Recent advancements in nonlinear nanophotonics are driven by the exploration of sharp resonances within high-index dielectric metasurfaces. In this work, we leverage doubly degenerate quasi-bound states in the continuum (quasi-BICs) to demonstrate the robust enhancement of third-harmonic generation (THG) in silicon metasurfaces. These quasi-BICs are governed by C 4 v symmetry and therefore can be equally excited with the pump light regardless of polarization. By tailoring the geometric parameters, we effectively control Q -factors and field confinement of quasi-BICs and thus regulate their resonantly enhanced THG process. A maximum THG conversion efficiency up to 1.03 × 10 –5 is recorded under a pump intensity of 5.85 GW/cm 2 . Polarization-independent THG profiles are further confirmed by mapping their signals across the polarization directions. This work establishes foundational strategies for the ultracompact design of robust and high-efficiency photon upconversion systems.

Topics & Concepts

Polarization (electrochemistry)Excited stateDegenerate energy levelsSecond-harmonic generationPhysicsNonlinear systemNonlinear opticsPhoton upconversionLinear polarizationPhotonDielectricOptoelectronicsOpticsAtomic physicsQuantum mechanicsExcitationChemistryPhysical chemistryLaserMetamaterials and Metasurfaces ApplicationsPlasmonic and Surface Plasmon ResearchAdvanced Antenna and Metasurface Technologies