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Adsorption Separation of Cr(VI) from a Water Phase Using Multiwalled Carbon Nanotube-Immobilized Ionic Liquids

Lihan Sun, Mengru Wang, Wei Li, Sha Luo, Yan Wu, Chunhui Ma, Shouxin Liu

2020ACS Omega27 citationsDOIOpen Access PDF

Abstract

were investigated by single-factor analysis. The results showed that the Cr(VI) removal rate was 52.14% and the adsorption capacity was 31.29 mg/g. The optimum adsorption conditions were as follows: initial Cr(VI) concentration, 60 mg/L; adsorbent dosage, 50 mg; pH 2.0; adsorption temperature 40 °C; and adsorption time, 200 min. Adsorption isotherm data fitted the Freundlich model, which indicates that the adsorption process was in line with the multimolecular layer adsorption theory. The Cr(VI) adsorption behaviors of the three adsorbents were consistent with a pseudo-second-order dynamic model. Thermodynamic analysis of the reaction systems was also performed. The Cr(VI) removal rates of MWCNTs-3, MWCNTs-OH-3, and MWCNTs-COOH-3 were 27.97, 9.39, and 7.34% lower than the initial removal rates after five cycles.

Topics & Concepts

AdsorptionThermogravimetric analysisIonic liquidFreundlich equationCarbon nanotubeFourier transform infrared spectroscopyChemistryTitrationX-ray photoelectron spectroscopyActivated carbonIonic strengthC4mimNuclear chemistryChemical engineeringMaterials scienceInorganic chemistryOrganic chemistryAqueous solutionNanotechnologyCatalysisEngineeringAdsorption and biosorption for pollutant removalAnalytical chemistry methods developmentExtraction and Separation Processes