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Density-functional tight-binding for phosphine-stabilized nanoscale gold clusters

Van‐Quan Vuong, Jenica Marie L. Madridejos, Bálint Aradi, Bobby G. Sumpter, Gregory F. Metha, Stephan Irle

2020Chemical Science26 citationsDOIOpen Access PDF

Abstract

We report a parameterization of the density-functional tight-binding (DFTB) method for the accurate prediction of molecular, electronic and vibrational structure of phosphine-ligated nanoscale gold clusters, metalloids, and gold surfaces.

Topics & Concepts

PhosphineNanoscopic scaleTight bindingDensity functional theoryChemical physicsMaterials scienceComputational chemistryElectronic structureNanotechnologyChemistryOrganic chemistryCatalysisNanocluster Synthesis and ApplicationsGold and Silver Nanoparticles Synthesis and ApplicationsMolecular Junctions and Nanostructures
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