Litcius/Paper detail

Phonon thermal Hall effect in a metallic spin ice

Taiki Uehara, Takumi Ohtsuki, Masafumi Udagawa, Satoru Nakatsuji, Yo Machida

2022Nature Communications35 citationsDOIOpen Access PDF

Abstract

Abstract It has become common knowledge that phonons can generate thermal Hall effect in a wide variety of materials, although the underlying mechanism is still controversial. We study longitudinal κ x x and transverse κ x y thermal conductivity in Pr 2 Ir 2 O 7 , which is a metallic analog of spin ice. Despite the presence of mobile charge carriers, we find that both κ x x and κ x y are dominated by phonons. A T / H scaling of κ x x unambiguously reveals that longitudinal heat current is substantially impeded by resonant scattering of phonons on paramagnetic spins. Upon cooling, the resonant scattering is strongly affected by a development of spin ice correlation and κ x x deviates from the scaling in an anisotropic way with respect to field directions. Strikingly, a set of the κ x x and κ x y data clearly shows that κ x y correlates with κ x x in its response to magnetic field including a success of the T / H scaling and its failure at low temperature. This remarkable correlation provides solid evidence that an indispensable role is played by spin-phonon scattering not only for hindering the longitudinal heat conduction, but also for generating the transverse response.

Topics & Concepts

Condensed matter physicsPhononScatteringAnisotropyHeat currentPhonon scatteringSpin (aerodynamics)ScalingPhysicsThermal conductivityParamagnetismThermal conductionMagnetic fieldSpinsTransverse planeMaterials scienceThermodynamicsOpticsQuantum mechanicsGeometryStructural engineeringEngineeringMathematicsAdvanced Condensed Matter PhysicsTopological Materials and PhenomenaMultiferroics and related materials