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Trifluoromethylthiolation, Trifluoromethylation, and Arylation Reactions of Difluoro Enol Silyl Ethers

Xingguo Jiang, Denise N. Meyer, Dominik Baran, Miguel A. Cortés González, Kálmán J. Szabó

2020The Journal of Organic Chemistry26 citationsDOIOpen Access PDF

Abstract

group, which can be combined with the high electrophilicity of the difluoroketone motif. The methodology could also be extended to difluoro homologation of the trifluoromethyl ketones using the Togni reagent. In addition, we presented a method for transition-metal-free arylation of difluoro enol silyl ethers based on hypervalent iodines.

Topics & Concepts

Hypervalent moleculeSilylationEnolTrifluoromethylationElectrophileChemistryMoietyTrifluoromethylReagentElectrophilic fluorinationOrganic chemistryAlkylCatalysisFluorine in Organic ChemistryInorganic Fluorides and Related Compounds
Trifluoromethylthiolation, Trifluoromethylation, and Arylation Reactions of Difluoro Enol Silyl Ethers | Litcius