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Amine‐Catalyzed Copper‐Mediated C−H Sulfonylation of Benzaldehydes via a Transient Imine Directing Group**

Joe I. Higham, James A. Bull

2022Angewandte Chemie International Edition36 citationsDOIOpen Access PDF

Abstract

Abstract Transient directing groups (TDGs) can provide a powerful means for C−H functionalization without requiring additional steps for directing group introduction and removal. We report the first use of a TDG in combination with copper to effect C−H functionalization. The regioselective copper mediated β−C(sp 2 )−H sulfonylation of aldehydes with sulfinate salts is accomplished using catalytic β‐alanine to form a transient imine. A broad range of sulfonylated benzaldehydes are prepared using copper fluoride as both copper source and oxidant, involving a [5,6] cupracyclic intermediate. γ‐( peri )‐Sulfonylation of napthyl and phenanthrenyl carboxaldehydes is achieved through [6,6] cupracyclic intermediates. Further derivatisation of the aldehyde products is demonstrated. Kinetic experiments and Hammett analysis suggest the turnover limiting step to be a concerted asynchronous C−H cleavage via a dearomative Wheland‐type transition state.

Topics & Concepts

Surface modificationImineCopperRegioselectivityAmine gas treatingChemistryCatalysisGroup (periodic table)Combinatorial chemistryOrganic chemistryPhysical chemistryCatalytic C–H Functionalization MethodsSulfur-Based Synthesis TechniquesSynthesis and Catalytic Reactions
Amine‐Catalyzed Copper‐Mediated C−H Sulfonylation of Benzaldehydes via a Transient Imine Directing Group** | Litcius