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Enantioselective Synthesis of Isoindolinone by Sequential Palladium-Catalyzed Aza-Heck/Suzuki Coupling Reaction

Lei Wang, Wenyu Zhang, Shuaijie Wu, Qing Wu, Ying Han, Chao‐Guo Yan, Guodong Zhang

2024Organic Letters10 citationsDOI

Abstract

-phenyl hydroxamic ethers with readily available arylboronic and alkenyl boronic acids. This protocol is enabled by a palladium catalyst paired with chiral phosphoramidite ligands, particularly under mild reaction conditions, yielding efficient and succinct synthetic routes to chiral isoindolinones with high enantioselectivity. Furthermore, this reaction exhibits excellent functional group compatibility and a rich diversity of subsequent transformations.

Topics & Concepts

ChemistryEnantioselective synthesisPalladiumHeck reactionCombinatorial chemistrySuzuki reactionCatalysisCoupling (piping)Organic chemistryMechanical engineeringEngineeringSynthesis and pharmacology of benzodiazepine derivativesCancer Treatment and PharmacologySynthetic Organic Chemistry Methods