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Exploring natural and accelerated carbonation of alkali-activated slag

Joonho Seo, Seunghee Park, Seunghee Park, G.M. Kim, Solmoi Park, Solmoi Park

2024Construction and Building Materials11 citationsDOIOpen Access PDF

Abstract

The present study explores the natural and accelerated carbonation of alkali-activated slag. Six different activators of NaOH, Na 2 SiO 3 , Na 2 CO 3 , Na 2 SO 4 , CaO or MgO were used to make alkali-activated slag samples, and samples were accelerated-carbonated for 28 days or naturally-carbonated for 2 years. The types of calcium carbonate formed after carbonation varied depending on the activator and the carbonation condition. The stability of hydrotalcite-like layered double hydroxide was found to be underestimated when exposed to accelerated carbonation conditions, thus requiring caution when testing the durability performance of these materials under such conditions. CaCO 3 and the highly crosslinked aluminosilicate gel were the predominant carbonation products in both accelerated and natural carbonation, with the effects on the Al local environment differing between the carbonation conditions.

Topics & Concepts

CarbonationSlag (welding)Natural (archaeology)Alkali metalEnvironmental scienceMetallurgyMaterials scienceChemistryGeologyComposite materialPaleontologyOrganic chemistryConcrete and Cement Materials ResearchMagnesium Oxide Properties and ApplicationsCO2 Sequestration and Geologic Interactions
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