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Plasma Promotes Dry Reforming Reaction of CH4 and CO2 at Room Temperature with Highly Dispersed NiO/γ-Al2O3 Catalyst

Shanshan Lin, Peng-Rui Li, Hui-Bo Jiang, Jian-Feng Diao, Zhong‐Ning Xu, Guo‐Cong Guo

2021Catalysts16 citationsDOIOpen Access PDF

Abstract

Plasma is an efficient method that can activate inert molecules such as methane and carbon dioxide in a mild environment to make them reactive. In this work, we have prepared an AE-NiO/γ-Al2O3 catalyst using an ammonia-evaporation method for plasma promoted dry reforming reaction of CO2 and CH4 at room temperature. According to the characterization data of XRD, H2-TPR, TEM, XPS, etc., the AE-NiO/γ-Al2O3 catalyst has higher dispersion, smaller particle size and stronger metal-support interaction than the catalyst prepared by the traditional impregnation method. In addition, the AE-NiO/γ-Al2O3 catalyst also exhibits higher activity in dry reforming reaction. This work provides a feasible reference experience for the research of plasma promoted dry reforming reaction catalysts at room temperature.

Topics & Concepts

Carbon dioxide reformingNon-blocking I/OCatalysisInertMaterials scienceChemical engineeringMethaneX-ray photoelectron spectroscopyDispersion (optics)SyngasChemistryOrganic chemistryEngineeringOpticsPhysicsCatalysts for Methane ReformingCatalytic Processes in Materials ScienceCarbon dioxide utilization in catalysis
Plasma Promotes Dry Reforming Reaction of CH4 and CO2 at Room Temperature with Highly Dispersed NiO/γ-Al2O3 Catalyst | Litcius