Litcius/Paper detail

Electrochemical Deoxygenative Thiolation of Preactivated Alcohols and Ketones

Feng Zhang, Yang Wang, Yi Wang, Yi Pan

2021Organic Letters37 citationsDOI

Abstract

This work describes an electrochemically promoted nickel-catalyzed deoxygenative thiolation of alcohols and ketones under mild conditions. Excellent substrate tolerance and good chemical yields can be achieved by graphene/nickel foam electrodes in an undivided cell. Further study to gain mechanistic insight into this electrochemical cross-coupling has been carried out.

Topics & Concepts

ChemistryElectrochemistryNickelSubstrate (aquarium)Combinatorial chemistryCatalysisElectrodeOrganic chemistryGeologyOceanographyPhysical chemistrySulfur-Based Synthesis TechniquesRadical Photochemical ReactionsCatalytic C–H Functionalization Methods