An experimental and computational look at the radiolytic degradation of TODGA and the effect on metal complexation
Ashleigh Kimberlin, Dominique Guillaumont, Sylvie Arpigny, B. Camès, Philippe Guilbaud, Georges Saint-Louis, Hitos Galán, Laurence Berthon
Abstract
A combination of Fukui function calculations with experimental characterization gives an improved understanding of the behaviour of TODGA solutions after radiolysis.
Topics & Concepts
ChemistryRadiolysisDegradation (telecommunications)MetalInorganic chemistryRadicalOrganic chemistryComputer scienceTelecommunicationsRadioactive element chemistry and processingNuclear Materials and PropertiesMolten salt chemistry and electrochemical processes