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A rapid and sensitive method for chiroptical sensing of α-amino acids <i>via</i> click-like labeling with <i>o</i> -phthalaldehyde and <i>p</i> -toluenethiol

Bo Li, Jie Zhang, Li Li, Gong Chen

2020Chemical Science28 citationsDOIOpen Access PDF

Abstract

group of analytes into an isoindole. The covalent labeling generates sensitive UV and CD readouts, both of which show an excellent linear relationship with the concentration of analytes. The high reactivity and the novel optical reporting mechanism allow fast and accurate measurement without background interference. The sensing assay works well for a remarkably broad range of analyte concentrations, with an unprecedented lower limit of 10 micromolar concentration.

Topics & Concepts

IsoindoleAnalyteChemistryO-PhthalaldehydeReagentCombinatorial chemistryCovalent bondLinear rangeDetection limitChromatographyDerivatizationStereochemistryHigh-performance liquid chromatographyOrganic chemistryMolecular Sensors and Ion DetectionLuminescence and Fluorescent MaterialsChemical Synthesis and Analysis
A rapid and sensitive method for chiroptical sensing of α-amino acids <i>via</i> click-like labeling with <i>o</i> -phthalaldehyde and <i>p</i> -toluenethiol | Litcius