Ultrafast, All Optically Reconfigurable, Nonlinear Nanoantenna
Eva A. A. Pogna, Michele Celebrano, Andrea Mazzanti, Lavinia Ghirardini, Luca Carletti, Giuseppe Marino, Andrea Schirato, Daniele Viola, P. Laporta, Costantino De Angelis, Giuseppe Leo, Giulio Cerullo, Marco Finazzi, Giuseppe Della Valle
Abstract
nanoscale engineering is a hot topic of research. Optical nanoantennas increase light-matter interaction and provide, simultaneously, a high throughput of the generated harmonics in the scattered light. However, nanoscale nonlinear optics has dealt so far with static or quasi-static configurations, whereas advanced applications would strongly benefit from high-speed reconfigurable nonlinear nanophotonic devices. Here we propose and experimentally demonstrate ultrafast all-optical modulation of the second harmonic (SH) from a single nanoantenna. Our design is based on a subwavelength AlGaAs nanopillar driven by a control femtosecond light pulse in the visible range. The control pulse photoinjects free carriers in the nanostructure, which in turn induce dramatic permittivity changes at the band edge of the semiconductor. This results in an efficient modulation of the SH signal generated at 775 nm by a second femtosecond pulse at the 1.55 μm telecommunications (telecom) wavelength. Our results can lead to the development of ultrafast, all optically reconfigurable, nonlinear nanophotonic devices for a broad class of telecom and sensing applications.