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A Nucleophilic Deprotection of Carbamate Mediated by 2-Mercaptoethanol

Thomas Scattolin, Tawfik Gharbaoui, Cheng‐yi Chen

2022Organic Letters13 citationsDOI

Abstract

Carbamates, typically used for the protection of amines, including Cbz, Alloc, and methyl carbamate, can be readily deprotected by treatment with 2-mercaptoethanol in the presence of potassium phosphate tribasic in N,N-dimethylacetamide at 75 °C. This nucleophilic deprotection protocol is superior to the standard hydrogenolysis or Lewis acid-mediated deprotection conditions for substrates bearing a functionality sensitive to these more traditional methods.

Topics & Concepts

ChemistryHydrogenolysisCarbamateNucleophileDimethylacetamideLewis acids and basesPotassiumOrganic chemistryCombinatorial chemistryCatalysisSolventChemical Synthesis and AnalysisChemical Synthesis and ReactionsAsymmetric Hydrogenation and Catalysis
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