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Effect of TiO2 and FeO on viscosity and structure of HIsmelt titanium-containing slag

Shushi Zhang, Zhenyang Wang, Jianliang Zhang, Peimin Guo, Dewen Jiang, Ruishuai Si

2023Ceramics International40 citationsDOIOpen Access PDF

Abstract

HIsmelt is considered one of the most promising processes for future vanadium-titanium magnetite smelting. In this study, we investigated the effects of TiO 2 and FeO on the viscosity and structure properties of HIsmelt titanium-containing slag using the rotating cylinder method, the Fourier Transform Infrared, and Raman. Experimental findings indicate a significant reduction in melting temperature with increasing TiO 2 content, accompanied by a rapid decrease in slag viscosity followed by a gradual increase, reaching a minimum at 30 wt% TiO 2 . The FeO content exerts minimal influence on slag viscosity and melting temperature. FTIR spectroscopy results reveal a gradual depolymerization of the [SiO 4 ] structure with the introduction of TiO 2 and FeO while having little influence on [AlO 4 ] and Si–O–Al structural changes. Raman spectroscopy results indicate an increase in Q 0 and a decrease in Q 1 and Q 2 with elevated TiO 2 and FeO content, leading to a reduction in the degree of polymerization (DOP) within the silicate structure and, consequently, lower slag viscosity. Maintaining FeO content within the range of 2–4% and TiO 2 content at approximately 30 % will be advantageous for industrial production.

Topics & Concepts

Slag (welding)Materials scienceTitaniumDepolymerizationViscosityFourier transform infrared spectroscopyRaman spectroscopyVanadiumMagnetiteSmeltingSilicatePolymerizationChemical engineeringMetallurgyComposite materialPolymerPolymer chemistryPhysicsEngineeringOpticsMetallurgical Processes and ThermodynamicsIron and Steelmaking ProcessesMetal Extraction and Bioleaching
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