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Mode of Action of Disinfection Chemicals on the Bacterial Spore Structure and Their Raman Spectra

Dmitry Malyshev, Tobias Dahlberg, Krister Wiklund, Per Ola Andersson, Sara Henriksson, Magnus Andersson

2021Analytical Chemistry61 citationsDOIOpen Access PDF

Abstract

spores treated with sporicidal agents such as chlorine dioxide, peracetic acid, and sodium hypochlorite using laser tweezers Raman spectroscopy. We also image treated spores using SEM and TEM to verify if we can correlate structural changes in the spores with changes to their Raman spectra. We found that over 30 min, chlorine dioxide did not change the Raman spectrum or the spore structure, peracetic acid showed a time-dependent decrease in the characteristic DNA/DPA peaks and ∼20% of the spores were degraded and collapsed, and spores treated with sodium hypochlorite showed an abrupt drop in DNA and DPA peaks within 20 min and some structural damage to the exosporium. Structural changes appeared in spores after 10 min, compared to the inactivation time of the spores, which is less than a minute. We conclude that vibrational spectroscopy provides powerful means to detect changes in spores but it might be problematic to identify if spores are live or dead after a decontamination procedure.

Topics & Concepts

SporePeracetic acidChemistrySodium hypochloriteChlorine dioxideHuman decontaminationDipicolinic acidRaman spectroscopyEndosporeMicrobiologyBiochemistryHydrogen peroxideInorganic chemistryBiologyOrganic chemistryOpticsPhysicsNuclear physicsBacillus and Francisella bacterial researchSpectroscopy Techniques in Biomedical and Chemical ResearchListeria monocytogenes in Food Safety