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First principle study of scandium-based novel ternary half Heusler ScXGe (X = Mn and Fe) alloys: insight into the spin-polarized structural, electronic, and magnetic properties

Hayat Ullah, Sadia Yasin, Kashif Safeen, Adeel Younus, Zeinhom M. El‐Bahy, Akif Safeen, Safaa N. Abdou, Mohamed M. Ibrahim

2024RSC Advances36 citationsDOIOpen Access PDF

Abstract

) to highlight the strong exchange-correlation interaction in these alloys. The structural parameter optimizations, whether ferromagnetic (FM) or nonmagnetic (NM), reveal that all ScXGe (where X = Mn, Fe) Heusler alloys attain their lowest ground state energy during FM optimization. The examination of the electronic properties of these alloys reveals their metallic character in both the spin-up and spin-down channels. The projected densities of states indicate that bonding is achieved through the hybridization of p-d and d-d states in all of the compounds. The investigation of the magnetic properties in ScXGe (where X = Mn, Fe) compounds indicates pronounced stability in their ferromagnetic state. Notably, the Curie temperatures for ScXGe (X = Mn, Fe) are determined to be 2177.02 K and 1656.09 K, respectively. The observation of metallic behavior and the strong ferromagnetic characteristics in ScXGe (X = Mn, Fe) half-Heusler alloys underscores their potential significance in the realm of spintronic devices. Consequently, our study serves as a robust foundation for subsequent experimental validation.

Topics & Concepts

ScandiumTernary operationDegenerate energy levelsCondensed matter physicsMaterials scienceSpintronicsSpin (aerodynamics)Ternary alloyCrystallographyAlloyChemistryPhysicsFerromagnetismMetallurgyThermodynamicsQuantum mechanicsComputer scienceProgramming languageHeusler alloys: electronic and magnetic propertiesMXene and MAX Phase MaterialsMagnetic and transport properties of perovskites and related materials