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Negative Differential Resistance with Ultralow Peak-to-Valley Voltage Difference in Td-WTe<sub>2</sub>/2H-MoS<sub>2</sub> Heterostructure

Shida Huo, Hengze Qu, Fanying Meng, Zhe Zhang, Zheyu Yang, Shengli Zhang, Xiaodong Hu, Enxiu Wu

2024Nano Letters106 citationsDOI

Abstract

Negative differential resistance (NDR) devices with a low peak-to-valley voltage difference (Δ V ) exhibit a high cut off frequency and low power consumption efficiency, which is significant for fabricating high-performance oscillators. However, achieving an ultralow Δ V is challenging. In this work, we report the first construction of an NDR device utilizing a van der Waals heterostructure composed of semimetallic Td-WTe 2 and semiconducting 2H-MoS 2 . Our findings reveal that the narrow energy region of the decreasing density of states (DOS) above the Fermi level of WTe 2 acts as a narrow band gap, facilitating type-III band alignment with MoS 2 and enabling band-to-band tunneling-based NDR transport. Notably, the NDR device exhibits an ultralow Δ V of approximately 0.01 V, which is at least an order of magnitude lower than previously reported values. This work not only introduces a new approach for NDR device fabrication but also provides new insights into the pivotal role of Td-WTe 2 in NDR transport.

Topics & Concepts

HeterojunctionMaterials scienceDifferential (mechanical device)Analytical Chemistry (journal)OptoelectronicsChemistryPhysicsThermodynamicsChromatography2D Materials and ApplicationsMXene and MAX Phase MaterialsPerovskite Materials and Applications
Negative Differential Resistance with Ultralow Peak-to-Valley Voltage Difference in Td-WTe<sub>2</sub>/2H-MoS<sub>2</sub> Heterostructure | Litcius