Litcius/Paper detail

Zeolite-Encaged Isolated Platinum Ions Enable Heterolytic Dihydrogen Activation and Selective Hydrogenations

Xin Deng, Bin Qin, Runze Liu, Xuetao Qin, Weili Dai, Guangjun Wu, Naijia Guan, Ding Ma, Landong Li

2021Journal of the American Chemical Society187 citationsDOI

Abstract

Understanding the unique behaviors of atomically dispersed catalysts and the origin thereof is a challenging topic. Herein, we demonstrate a facile strategy to encapsulate Ptδ+ species within Y zeolite and reveal the nature of selective hydrogenation over a Pt@Y model catalyst. The unique configuration of Pt@Y, namely atomically dispersed Ptδ+ stabilized by the surrounding oxygen atoms of six-membered rings shared by sodalite cages and supercages, enables the exclusive heterolytic activation of dihydrogen over Ptδ+···O2– units, resembling the well-known classical Lewis pairs. The charged hydrogen species, i.e., H+ and Hδ−, are active reagents for selective hydrogenations, and therefore, the Pt@Y catalyst exhibits remarkable performance in the selective hydrogenation of α,β-unsaturated aldehydes to unsaturated alcohols and of nitroarenes to arylamines.

Topics & Concepts

HeterolysisChemistryCatalysisZeolitePlatinumSodaliteMolecular sieveHydrogenReagentIonLewis acids and basesInorganic chemistryPhotochemistryOrganic chemistryAsymmetric Hydrogenation and CatalysisNanomaterials for catalytic reactionsCatalysis and Hydrodesulfurization Studies