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<i>In situ</i> formation of circular and branched oligomers in a localized high concentration electrolyte at the lithium-metal solid electrolyte interphase: a hybrid <i>ab initio</i> and reactive molecular dynamics study

Yue Liu, Qintao Sun, Peiping Yu, Bingyun Ma, Hao Yang, Jiayi Zhang, Miao Xie, Tao Cheng

2021Journal of Materials Chemistry A19 citationsDOI

Abstract

Developing advanced electrolytes has been considered as a promising approach to stabilize the lithium metal anode via the formation of a stable solid electrolyte interphase (SEI) that can protect the Li anode to enable long-term cycling stability.

Topics & Concepts

InterphaseElectrolyteAnodeLithium metalLithium (medication)Materials scienceMetalChemical engineeringFast ion conductorInorganic chemistryChemistryElectrodePhysical chemistryMetallurgyGeneticsBiologyEngineeringEndocrinologyMedicineAdvancements in Battery MaterialsAdvanced Battery Materials and TechnologiesAdvanced Battery Technologies Research
<i>In situ</i> formation of circular and branched oligomers in a localized high concentration electrolyte at the lithium-metal solid electrolyte interphase: a hybrid <i>ab initio</i> and reactive molecular dynamics study | Litcius