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Gate-tunable Intrinsic Anomalous Hall Effect in Epitaxial MnBi<sub>2</sub>Te<sub>4</sub> Films

Shanshan Liu, Jie-Xiang Yu, Enze Zhang, Zihan Li, Qiang Sun, Yong Zhang, Liwei Cao, Lun Li, Minhao Zhao, Pengliang Leng, Xiangyu Cao, Ang Li, Jin Zou, Xufeng Kou, Jiadong Zang, Faxian Xiu

2023Nano Letters27 citationsDOI

Abstract

The anomalous Hall effect (AHE) is an important transport signature revealing topological properties of magnetic materials and their spin textures. Recently, MnBi 2 Te 4 has been demonstrated to be an intrinsic magnetic topological insulator. However, the origin of its intriguing AHE behaviors remains elusive. Here, we demonstrate the Berry curvature-dominated intrinsic AHE in wafer-scale MnBi 2 Te 4 films. By applying back-gate voltages, we observe an ambipolar conduction and n–p transition in ∼7-layer MnBi 2 Te 4, where a quadratic relation between the AHE resistance and longitudinal resistance suggests its intrinsic AHE nature. In particular, for ∼3-layer MnBi 2 Te 4, the AHE sign can be tuned from pristine negative to positive. First-principles calculations unveil that such an AHE reversal originated from the competing Berry curvature between oppositely polarized spin-minority-dominated surface states and spin-majority-dominated inner bands. Our results shed light on the underlying physical mechanism of the intrinsic AHE and provide new perspectives for the unconventional sign-tunable AHE.

Topics & Concepts

Berry connection and curvatureCondensed matter physicsHall effectAmbipolar diffusionTopological insulatorSpin (aerodynamics)Materials sciencePhysicsMagnetic fieldGeometric phaseElectronQuantum mechanicsThermodynamicsTopological Materials and PhenomenaAdvanced Condensed Matter PhysicsMagnetic properties of thin films