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Molecular-Level Insight into the Interfacial Reactivity and Ionic Conductivity of a Li-Argyrodite Li<sub>6</sub>PS<sub>5</sub>Cl Solid Electrolyte at Bare and Coated Li-Metal Anodes

Andrey A. Golov, Javier Carrasco

2021ACS Applied Materials & Interfaces49 citationsDOIOpen Access PDF

Abstract

as the most suitable coating to partially prevent the electrolyte degradation while keeping a relatively low interfacial resistance. These findings shed light on the interface chemistry of sulfide-based electrolytes in contact with Li metal and pave the way for rationalizing further computational and experimental studies in the field.

Topics & Concepts

Materials scienceElectrolyteIonic conductivityAnodeFast ion conductorConductivityMetalIonic bondingReactivity (psychology)SulfideChemical engineeringChemical physicsIonInorganic chemistryElectrodePhysical chemistryChemistryMetallurgyOrganic chemistryAlternative medicineMedicineEngineeringPathologyAdvanced Battery Materials and TechnologiesAdvancements in Battery MaterialsAdvanced Battery Technologies Research
Molecular-Level Insight into the Interfacial Reactivity and Ionic Conductivity of a Li-Argyrodite Li<sub>6</sub>PS<sub>5</sub>Cl Solid Electrolyte at Bare and Coated Li-Metal Anodes | Litcius