Spatial acid–base–Pd triple-sites of a hierarchical core–shell structure for three-step tandem reaction
Jian Wu, Ganggang Chang, You-Qing Peng, Xiaochen Ma, Shan‐Chao Ke, Si‐Ming Wu, Yuxuan Xiao, Ge Tian, Tao Xia, Xiaoyu Yang
Abstract
Spatial catalytic acid-base-Pd triple-sites of a hierarchical core-shell structure have been successfully constructed for a three-step reaction, and exhibited excellent catalytic activity and stability. A catalytic mechanism has been systematically studied via single one- and two-step reactions, and possible molecular reactions have been proposed.
Topics & Concepts
CatalysisTandemCore (optical fiber)ChemistryBase (topology)Reaction conditionsShell (structure)Combinatorial chemistryMaterials scienceOrganic chemistryMathematical analysisMathematicsComposite materialAsymmetric Hydrogenation and CatalysisNanomaterials for catalytic reactionsMetal-Organic Frameworks: Synthesis and Applications