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Emergence of superconductivity in doped multiorbital Hubbard chains

Niravkumar D. Patel, Nitin Kaushal, Alberto Nocera, Gonzalo Álvarez, Elbio Dagotto

2020npj Quantum Materials20 citationsDOIOpen Access PDF

Abstract

Abstract We introduce a variational state for one-dimensional two-orbital Hubbard models that intuitively explains the recent computational discovery of pairing in these systems when hole doped. Our ansatz is an optimized linear superposition of Affleck–Kennedy–Lieb–Tasaki valence-bond states, rendering the combination a valence-bond liquid dubbed orbital resonant valence bond. We show that the undoped (one-electron/orbital) quantum state of two sites coupled into a global spin singlet is exactly written employing only spin-1/2 singlets linking orbitals at nearest-neighbor sites. Generalizing to longer chains defines our variational state visualized geometrically expressing our chain as a two-leg ladder, with one orbital per leg. As in Anderson’s resonating valence-bond state, our undoped variational state contains preformed singlet pairs that via doping become mobile, leading to superconductivity. Doped real materials with one-dimensional substructures, two near-degenerate orbitals, and intermediate Hubbard U / W strengths— W the carrier’s bandwidth—could realize spin-singlet pairing if on-site anisotropies are small. If these anisotropies are robust, spin-triplet pairing emerges.

Topics & Concepts

PairingValence bond theorySinglet statePhysicsAtomic orbitalHubbard modelCondensed matter physicsGeneralized valence bondDegenerate energy levelsSuperconductivityAnsatzGround stateModern valence bond theoryQuantum mechanicsChemistryElectronExcited statePhysics of Superconductivity and MagnetismAdvanced Condensed Matter PhysicsIron-based superconductors research
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