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A rotational investigation of the three isomeric forms of cyanoethynylbenzene (HCC-C<sub>6</sub>H<sub>4</sub>-CN): benchmarking experiments and calculations using the “Lego brick” approach

J.-T. Spaniol, Kin Long Kelvin Lee, Olivier Pirali, Cristina Puzzarini, Marie‐Aline Martin‐Drumel

2023Physical Chemistry Chemical Physics13 citationsDOIOpen Access PDF

Abstract

, 9904-9916]. From these assignments, accurate spectroscopic (rotational and centrifugal distortion) constants have been derived: for all species and all observed vibrational states, predicted rotational constants show relative accuracy better than 0.1%, and often of the order of 0.01%, compared to the experimental values. The present work hence further validates the use of the "Lego brick" approach for predicting spectroscopic constants with high precision.

Topics & Concepts

BenchmarkingBrickComputational chemistryChemistryNanotechnologyMaterials scienceComposite materialMarketingBusinessMolecular Spectroscopy and StructureAdvanced Chemical Physics StudiesAstrophysics and Star Formation Studies