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Efficient conversion of carbohydrates into 5‐hydroxymethylfurfural using choline chloride-based deep eutectic solvents

Dung Kim Thi Ngo, Trinh Hao Nguyen, Phat Ngoc Nguyen, Hai Truong Nguyen, Trinh Ngoc Thi Huynh, Ha Bich Phan, Phuong Hoang Tran

2023Heliyon12 citationsDOIOpen Access PDF

Abstract

In this study, the conversion of monosaccharides to 5-hydroxymethylfurfural (5-HMF) using different deep eutectic solvents (DESs) was investigated in various conditions. Among all the investigated DESs, [ChCl][trichloroacetic acid], based on choline chloride and trichloroacetic acid with the ratio 1:1, showed the highest catalytic activity. A maximum 5-HMF yield was 82 % for 1 h at 100 °C using [ChCl][trichloroacetic acid] as a catalyst from fructose. [ChCl][trichloroacetic acid] could be recovered and reused three times with a slight loss in activity. Our work demonstrated the low-cost and effective method for the synthesis of 5-HMF from carbohydrates.

Topics & Concepts

Choline chlorideTrichloroacetic acidChemistryYield (engineering)CatalysisMonosaccharideFructoseEutectic systemOrganic chemistryChlorideNuclear chemistryChromatographyMaterials scienceMetallurgyAlloyCatalysis for Biomass ConversionSupercapacitor Materials and FabricationMesoporous Materials and Catalysis
Efficient conversion of carbohydrates into 5‐hydroxymethylfurfural using choline chloride-based deep eutectic solvents | Litcius