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Self-Adjuvanting Lipoprotein Conjugate αGalCer-RBD Induces Potent Immunity against SARS-CoV-2 and its Variants of Concern

Jian Wang, Yu Wen, Shihao Zhou, Haiwei Zhang, Xiaoqian Peng, Ruyan Zhang, Xuguang Yin, Hong Qiu, Rui Gong, Guang‐Fu Yang, Jun Guo

2022Journal of Medicinal Chemistry41 citationsDOI

Abstract

Safe and effective vaccines against severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2) and its variants are the best approach to successfully combat the COVID-19 pandemic. The receptor-binding domain (RBD) of the viral spike protein is a major target to develop candidate vaccines. α-Galactosylceramide (αGalCer), a potent invariant natural killer T cell (iNKT) agonist, was site-specifically conjugated to the N-terminus of the RBD to form an adjuvant–protein conjugate, which was anchored on the liposome surface. This is the first time that an iNKT cell agonist was conjugated to the protein antigen. Compared to the unconjugated RBD/αGalCer mixture, the αGalCer-RBD conjugate induced significantly stronger humoral and cellular responses. The conjugate vaccine also showed effective cross-neutralization to all variants of concern (B.1.1.7/alpha, B.1.351/beta, P.1/gamma, B.1.617.2/delta, and B.1.1.529/omicron). These results suggest that the self-adjuvanting αGalCer-RBD has great potential to be an effective COVID-19 vaccine candidate, and this strategy might be useful for designing various subunit vaccines.

Topics & Concepts

ChemistryConjugateImmunityVirologyImmunologyImmune systemMedicineMathematicsMathematical analysisinterferon and immune responsesImmune cells in cancerNanoplatforms for cancer theranostics