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Pyrene-based fluorescent Ru(<scp>ii</scp>)-arene complexes for significant biological applications: catalytic potential, DNA/protein binding, two photon cell imaging and<i>in vitro</i>cytotoxicity

Pragti Pragti, Bidyut Kumar Kundu, Shrish Nath Upadhyay, Nilima Sinha, Rakesh Ganguly, Ivo Grabchev, Srimanta Pakhira, Suman Mukhopadhyay

2022Dalton Transactions24 citationsDOI

Abstract

proteins (HSA and BSA) and CT-DNA. The density functional theory (DFT-D) method has been employed in the present study to know the interaction between DNA and complexes by calculating the HOMO and LUMO energy. A plausible mechanism for NADH oxidation has also been explored and the DFT calculations are found to be in accord with the experimental observation. Furthermore, we have investigated intracellular reactive oxygen species (ROS) generation capabilities in the MCF7 breast cancer cell line. The Hoechst/PI dual staining method confirmed the apoptosis mode of cell death. Meanwhile, complexes 1-4 show capabilities to prevent the metastasis phase of cancer cells by inhibiting cell migration.

Topics & Concepts

RutheniumChemistryHeLaMTT assayFluorescenceStereochemistryLigand (biochemistry)DenticityPhotochemistryCatalysisCrystallographyMedicinal chemistryCrystal structureIn vitroOrganic chemistryReceptorQuantum mechanicsBiochemistryPhysicsMetal complexes synthesis and propertiesClick Chemistry and ApplicationsFerrocene Chemistry and Applications
Pyrene-based fluorescent Ru(<scp>ii</scp>)-arene complexes for significant biological applications: catalytic potential, DNA/protein binding, two photon cell imaging and<i>in vitro</i>cytotoxicity | Litcius