Charge and spin communication between dual metal single-atom sites on C<sub>2</sub>N sheets: regulating electronic spin moments of Fe atoms for N<sub>2</sub>activation and reduction
Yuqin Zhang, Xiaohang Wang, Tianyong Liu, Qian Dang, Ling Zhu, Yi Luo, Jun Jiang, Shaobin Tang
Abstract
The charge and spin communication constructed between dual single-metal atom sites on C 2 N sheets significantly regulated the electronic spin moments of Fe atom active sites, and thus boosted electrochemical N 2 reduction to NH 3 .
Topics & Concepts
Atom (system on chip)Spin (aerodynamics)MetalCharge (physics)Atomic physicsReduction (mathematics)Materials scienceDual (grammatical number)ElectrochemistryChemistryCrystallographyPhysicsPhysical chemistryElectrodeMetallurgyQuantum mechanicsComputer scienceLiteratureThermodynamicsMathematicsGeometryEmbedded systemArtAmmonia Synthesis and Nitrogen ReductionAdvanced Photocatalysis TechniquesCatalytic Processes in Materials Science