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Room-temperature processed high-quality SnO <sub>2</sub> films by oxygen plasma activated e-beam evaporation

Jiankang Li, Lutao Li, Weiyuan Chen, Qinghua Yi, Guifu Zou

2020Nanotechnology12 citationsDOI

Abstract

Abstract Recently, SnO 2 is considered to be one of the most promising materials as electron transport layer in perovskite solar cells (PSCs). Low-temperature processed SnO 2 films are crucial for SnO 2 -based PSCs and flexible devices. However, it is difficult to prepare stoichiometric SnO 2 films by e-beam evaporation at low-temperature. Herein, SnO 2 films are fabricated by oxygen plasma activated e-beam evaporation technique at room-temperature. Oxygen plasma shows strong oxidation activity, which is essential to adjust the stoichiometry of SnO x in the evaporation process. The SnO 2 films exhibit uniformity ( R q = 3.05 nm), high transmittance ( T &gt; 90%), high hall mobility ( μ e = 10.8 cm 2 V − 1 s −1 ) and good hydrophilic (water contact angle =19°). This work will promote the application of SnO 2 films in PSCs and flexible devices.

Topics & Concepts

Materials scienceEvaporationElectron beam physical vapor depositionStoichiometryTransmittanceOxygenPerovskite (structure)Layer (electronics)PlasmaAnalytical Chemistry (journal)Thin filmOptoelectronicsNanotechnologyChemical engineeringOrganic chemistryChemistryEngineeringQuantum mechanicsPhysicsChromatographyThermodynamicsPerovskite Materials and ApplicationsZnO doping and propertiesGas Sensing Nanomaterials and Sensors
Room-temperature processed high-quality SnO <sub>2</sub> films by oxygen plasma activated e-beam evaporation | Litcius